Assembly of CuIn(1-x)Ga(x)S2 nanorods into highly ordered 2D and 3D superstructures.
Identifieur interne : 000F87 ( Main/Exploration ); précédent : 000F86; suivant : 000F88Assembly of CuIn(1-x)Ga(x)S2 nanorods into highly ordered 2D and 3D superstructures.
Auteurs : RBID : pubmed:22765274English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Copper, Gallium, Indium, Macromolecular Substances, Selenium.
- chemistry : Metal Nanoparticles.
- methods : Crystallization.
- ultrastructure : Metal Nanoparticles.
- Materials Testing, Molecular Conformation, Particle Size, Surface Properties.
Abstract
Here, we report self- and directed assembly of CuIn(1-x)Ga(x)S(2) (CIGS) nanorods into highly ordered 2D and 3D superstructures. The assembly protocol is dictated by the ligand environment and is hence chemically tunable. Thiol capped nanorods spontaneously assemble into 3D aligned nanorod clusters over a period of hours with end to end and side to side order. These clusters can be disassembled by ligand exchange with an amine and subsequently reassembled either at a substrate interface or as free floating 2D sheets by directed assembly protocols. This dimensional control of CIGS nanorod assembly, extending over device scale areas with high degrees of order, is highly attractive for applications utilizing these important quaternary photoabsorbers.
DOI: 10.1021/nn301999b
PubMed: 22765274
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The assembly protocol is dictated by the ligand environment and is hence chemically tunable. Thiol capped nanorods spontaneously assemble into 3D aligned nanorod clusters over a period of hours with end to end and side to side order. These clusters can be disassembled by ligand exchange with an amine and subsequently reassembled either at a substrate interface or as free floating 2D sheets by directed assembly protocols. This dimensional control of CIGS nanorod assembly, extending over device scale areas with high degrees of order, is highly attractive for applications utilizing these important quaternary photoabsorbers.</div></front></TEI><pubmed><MedlineCitation Owner="NLM" Status="MEDLINE"><PMID Version="1">22765274</PMID><DateCreated><Year>2012</Year><Month>08</Month><Day>28</Day></DateCreated><DateCompleted><Year>2013</Year><Month>01</Month><Day>03</Day></DateCompleted><DateRevised><Year>2013</Year><Month>11</Month><Day>21</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1936-086X</ISSN><JournalIssue CitedMedium="Internet"><Volume>6</Volume><Issue>8</Issue><PubDate><Year>2012</Year><Month>Aug</Month><Day>28</Day></PubDate></JournalIssue><Title>ACS nano</Title><ISOAbbreviation>ACS Nano</ISOAbbreviation></Journal><ArticleTitle>Assembly of CuIn(1-x)Ga(x)S2 nanorods into highly ordered 2D and 3D superstructures.</ArticleTitle><Pagination><MedlinePgn>6977-83</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/nn301999b</ELocationID><Abstract><AbstractText>Here, we report self- and directed assembly of CuIn(1-x)Ga(x)S(2) (CIGS) nanorods into highly ordered 2D and 3D superstructures. The assembly protocol is dictated by the ligand environment and is hence chemically tunable. Thiol capped nanorods spontaneously assemble into 3D aligned nanorod clusters over a period of hours with end to end and side to side order. These clusters can be disassembled by ligand exchange with an amine and subsequently reassembled either at a substrate interface or as free floating 2D sheets by directed assembly protocols. This dimensional control of CIGS nanorod assembly, extending over device scale areas with high degrees of order, is highly attractive for applications utilizing these important quaternary photoabsorbers.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Singh</LastName><ForeName>Ajay</ForeName><Initials>A</Initials><Affiliation>Materials and Surface Science Institute and Department of Chemical and Environmental Sciences,University of Limerick, Limerick, Ireland.</Affiliation></Author><Author ValidYN="Y"><LastName>Coughlan</LastName><ForeName>Claudia</ForeName><Initials>C</Initials></Author><Author ValidYN="Y"><LastName>Laffir</LastName><ForeName>Fathima</ForeName><Initials>F</Initials></Author><Author ValidYN="Y"><LastName>Ryan</LastName><ForeName>Kevin M</ForeName><Initials>KM</Initials></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType>Journal Article</PublicationType><PublicationType>Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2012</Year><Month>07</Month><Day>12</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Nano</MedlineTA><NlmUniqueID>101313589</NlmUniqueID><ISSNLinking>1936-0851</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance>Macromolecular Substances</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance>copper indium diselenide</NameOfSubstance></Chemical><Chemical><RegistryNumber>045A6V3VFX</RegistryNumber><NameOfSubstance>Indium</NameOfSubstance></Chemical><Chemical><RegistryNumber>789U1901C5</RegistryNumber><NameOfSubstance>Copper</NameOfSubstance></Chemical><Chemical><RegistryNumber>CH46OC8YV4</RegistryNumber><NameOfSubstance>Gallium</NameOfSubstance></Chemical><Chemical><RegistryNumber>H6241UJ22B</RegistryNumber><NameOfSubstance>Selenium</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName MajorTopicYN="N">Copper</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Crystallization</DescriptorName><QualifierName MajorTopicYN="N">methods</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Gallium</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Indium</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Macromolecular Substances</DescriptorName><QualifierName MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Materials Testing</DescriptorName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Metal Nanoparticles</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName><QualifierName MajorTopicYN="Y">ultrastructure</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Molecular Conformation</DescriptorName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Particle Size</DescriptorName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Selenium</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Surface Properties</DescriptorName></MeshHeading></MeshHeadingList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="aheadofprint"><Year>2012</Year><Month>7</Month><Day>12</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2012</Year><Month>7</Month><Day>7</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2012</Year><Month>7</Month><Day>7</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2013</Year><Month>1</Month><Day>4</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="doi">10.1021/nn301999b</ArticleId><ArticleId IdType="pubmed">22765274</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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